Environmental Monitoring Programs and Equipment Flashcards
What are the purposes of environmental monitoring?
- Measure and/or reconstruct (estimate) human population doses
- Determine radiological impact of a facility
- Detect and quantify accidental off-site radionuclide releases
- Meet specific license requirements
- Obtain pathway data to refine models
- Study air and water mixing patterns
Define
Pathway
(Environmental Monitoring)
Any route that radioactivity can follow in passing from a licensed facility to a person in the general population.
Define
Critical pathway
(Environmental Monitoring)
The route taken by a critical nuclide from point of release to body entry.
Compare and Contrast
Preoperational vs. and Postoperational Monitoring Programs
Preoperational Monitoring Program
- Put in place prior to the use of radioactivity at the site, and typically run for one year.
- Comprehensiveness ⇒ Determines a baseline analysis of environmental radioactivity over any possible areas of concern.
Postoperational Monitoring Program
- Sensitivity ⇒ Corresponds to a concentration of 1% to 10% of the applicable limits set for by federal or state radiation protection standards.
- Selectivity ⇒ Ability to select the radionuclide out of background.
Define
Critical nuclide
(Environmental Monitoring)
Those nuclei which cause the largest dose contribution to the actual population at risk near the facility.
What are the objectives of a preoperational monitoring program?
- Locate radiation anomalies
- Document ambient levels
- Identify critical nuclides and pathways
- Document seasonal meteorology patterns
What questions are to be answered by a preoperational monitoring program?
- What radioisotopes should be measured?
- Where should the samplers be located?
- How often should a sample be collected?
- Which equation is used to calculate population dose?
What is this plume pattern?
Looping
What is this plume pattern?
Coning
What is this plume pattern?
Fanning
What is this plume pattern?
Lofting
What is this plume pattern?
Fumigation
What are two practical techniques to overcome radon interference in environmental alpha monitors?
- Introduce a delay time between sample collection and counting to account for the short half-life of radon and its daughters.
- Use a detector such as a surface barrier diodide which have excellent energy resolution. Then use a single channel pulse height analyzer to eliminate the interference of the alphas particular to radon.
What questions need to be addressed in setting up a program to monitor the environmental levels of radioactivity?
- Which isotopes?
- Collection frequency?
- Sampling location?
- Sample preparation?
- Sampling medium?
- Counting equipment?
- Sample size?
- Calculational model?
How are environmental levels of external gamma radiation (“direct radiation”) measured?
- Using thermoluminescent dosimeters.
- Calcium fluoride and calcium sulphate TLDs are commonly used which can measure doses below 1 mrem per month.
What is a good TLD for environemental monitoring that represents human tissue?
- Use a carbon-doped aluminum oxide (Al2O3:C) phosphor which has an effective atomic number of 10.2. This is much closer to 7.5 than calcium phosphors.
- It has maximum fading of 10% in three months at extreme environmental temperatures, with no fading at room temperature for up to 9 months.
- Minimum detectable dose is 0.1 mrem.
How do you measure real time “direct exposure” gamma radiation?
- Use a pressurized ion chamber.
- Fill gas is pressurized to 600 psi with argon gas.
- The extra loading of gas molecules makes the chamber more sensitive.
- It can then detect a gamma ray background of as little as 1 mrem per year.
- This is good for plume detection.
What are some techniques and examples for monitoring airborne particulates?
- Sedimentation (Flypaper)
- Inertial Separation (Cascade Impactor)
- Filtration (High Volume Sampler)
- Electrostasis (Precipitator)
What are two factors to consider in operating a filter sampler?
- The accumulation of nonradioactive material on the filter element as time passes (dust loading). Problem in dusty environments.
- Change in efficiency of a filter matrix as the airflow velocity changes.
Graph
Collection Efficiency vs. Incoming Particle Velocity
(in reference to Air Filter Sampler for Environmental Monitoring)
Define
Stack sampling
- Sampling of particulates in a moving air stream.
- A stack is a vent pipe or duct carrying a stream of air molecules and particulates, possibly for release into the enviornment.
- If the particulates can possibly be radioactive their concentration must be measured before release.
Why would a stack monitor have a logarithmic readout?
- To allow coverage of levels from below background to disaster concentrations without range switching.
- A 30-day strip chart recorder gives a continuious record and makes it possible to calculate the amount of radioactivity released during any kind of evolution.
What are three considerations for a stack sampling?
- Type of nozzle
- The placement of the nozzle in the air stream
- The transport of the particulates to your collection point.
What design criteria must the nozzle meet?
(in reference to Stack Sampling)
- The nozzle must be designed to meet the conditions of isokinetic sampling.
- These conditions are met if the velocity of the air steam entering the nozzle is exactly equal to the velocity in the duct at the sampling point.
Define
Adsorption vs. Absorption
- Adsorption is the process in which atoms, ions, or molecules from a substance (it could be gas, liquid or dissolved solid) adhere to a surface of the adsorbent.
- Absorption is the process in which a fluid is dissolved by a liquid or a solid (absorbent).
What are some air sampling techniques for gases and examples?
- Continuous Flow (Stack Monitor)
- Grab Sample (Lucas Cell)
- Adsorption (Charcoal Canister)
- Condensation (Tritium Monitor)
How is a DAC value generated?
DAC (μCi mL-1) = ALI (μCi) ÷ 2.4 x 109 mL
- 2.4 x 109 mL is derived from the total volume of air (2,400 m3) breathed during a 2000 hour work year.
Define
Derived Air Concentration (DAC)
- If the air concentration is exactly equal to the DAC for one year, a worker will just reach the legal intake of radioactivity, one ALI, on December 31st.
- A worker not receiving any other radiation doses except by inhalation would be allowed a cumulative exposure of 2,000 DAC-hours in one working year.
What is an inexpensive method for screening houses for radon levels?
- A charcoal canister (3” in diameter and 1” high).
- A hole in the lid is covered by a “diffusion barrier” to increase the average sampling time, and holds about 25 grams of activated charcoal.
- Over the course of several days’ exposure, radon gas diffuses into the canister and adsorbs onto the charcoal.
- At the end of the exposure period, the canister is resealed and mailed back to an analytical lab for counting.
What are the alpha emissions from the 222Rn decay chain?
222Rn → 218Po
218Po → 214Pb
// 214Pb → 214Bi → 214Po (beta decay)
214Po → 210Pb
// 210Pb → 210Bi → 210Po (beta decay)
210Po → 206Pb (stable)
Define
Working level
- Any combination of short-lived radon daughters in one liter of air that will result in the emission of 1.3 x 105 MeV of potential alpha energy.
- If radon gas was present at a concentration of 100 pCi L-1, and if the daughter products were all in equilibrium, then the decay through the first 4 daughters would release exactly 1.3 x 105 MeV of alpha particle energy.
- The DAC for Rn-222 is 1/3 the working level.
How does an electret chamber work when measuring for radon?
- An electret is a material that can hold a permanent electrostatic charge.
- A teflon disk holds a charge through both humidity and temperature changes.
- Radon diffuses into a chamber containing the electret and the ionization caused by the radon gas decays and cancels some of the electrostatic charge on the positively charged electret.
- The surface voltage of the electret is measured before and after radon exposure.
- The voltage drop reveals the average radon concentration.
- Can be reused (cost is low) and insensitive to humidity and temperature.
NRC Regulatory Guide 1.97
What 3 levels of radioiondine monitoring are required?
- Reactor plant ⇒ The inplant air must be sampled during normal operations.
- Environmental ⇒ The environs outside the plant must be sampled periodicially.
- Accident monitoring ⇒ The plant must have special high range instruments available for post-accident monitoring.
How is routine monitoring accomplished for radioiodine?
- Sucking air through a collection medium with a high or low volume sampler.
- The collection medium is activated charcoal or silver impregnated zeolite.
- Charcoal cartidges are several times cheaper.
NRC Regulatory Guide 1.97
Monitoring equipment must be able to detect radioiodine in what range?
10-9 to 10-3 µCi cm-3
How do you accomplish tritium air sampling?
- Suck ambient air through an ioniziation chamber.
- Due to the very low energy of the tritium betas, a very sensitive electrometer circuit must be used to detect the tiny current produced inside the chamber by tritium decays.